Reversible switching of ultrastrong light-molecule coupling

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Reversible switching of ultrastrong light-molecule coupling. / Schwartz, T; Hutchison, J A; Genet, C; Ebbesen, T W.

In: Physical Review - Index, Vol. 106, 13.05.2011, p. 196405.

Research output: Contribution to journalJournal articleResearchpeer-review

Harvard

Schwartz, T, Hutchison, JA, Genet, C & Ebbesen, TW 2011, 'Reversible switching of ultrastrong light-molecule coupling', Physical Review - Index, vol. 106, pp. 196405. https://doi.org/10.1103/PhysRevLett.106.196405

APA

Schwartz, T., Hutchison, J. A., Genet, C., & Ebbesen, T. W. (2011). Reversible switching of ultrastrong light-molecule coupling. Physical Review - Index, 106, 196405. https://doi.org/10.1103/PhysRevLett.106.196405

Vancouver

Schwartz T, Hutchison JA, Genet C, Ebbesen TW. Reversible switching of ultrastrong light-molecule coupling. Physical Review - Index. 2011 May 13;106:196405. https://doi.org/10.1103/PhysRevLett.106.196405

Author

Schwartz, T ; Hutchison, J A ; Genet, C ; Ebbesen, T W. / Reversible switching of ultrastrong light-molecule coupling. In: Physical Review - Index. 2011 ; Vol. 106. pp. 196405.

Bibtex

@article{987cfd7e3e1a499b9d0f058bc157dd7c,
title = "Reversible switching of ultrastrong light-molecule coupling",
abstract = "We demonstrate that photochromic molecules enable switching from the weak- to ultrastrong-coupling regime reversibly, by using all-optical control. This switch is achieved by photochemically inducing conformational changes in the molecule. Remarkably, a Rabi splitting of 700 meV is measured at room temperature, corresponding to 32% of the molecular transition energy. A similar coupling strength is demonstrated in a plasmonic structure. Such systems present a unique combination of coupling strength and functional capacities.",
author = "T Schwartz and Hutchison, {J A} and C Genet and Ebbesen, {T W}",
year = "2011",
month = may,
day = "13",
doi = "10.1103/PhysRevLett.106.196405",
language = "English",
volume = "106",
pages = "196405",
journal = "Physical Review - Index",
issn = "0094-0003",
publisher = "New York, American Physical Society.",

}

RIS

TY - JOUR

T1 - Reversible switching of ultrastrong light-molecule coupling

AU - Schwartz, T

AU - Hutchison, J A

AU - Genet, C

AU - Ebbesen, T W

PY - 2011/5/13

Y1 - 2011/5/13

N2 - We demonstrate that photochromic molecules enable switching from the weak- to ultrastrong-coupling regime reversibly, by using all-optical control. This switch is achieved by photochemically inducing conformational changes in the molecule. Remarkably, a Rabi splitting of 700 meV is measured at room temperature, corresponding to 32% of the molecular transition energy. A similar coupling strength is demonstrated in a plasmonic structure. Such systems present a unique combination of coupling strength and functional capacities.

AB - We demonstrate that photochromic molecules enable switching from the weak- to ultrastrong-coupling regime reversibly, by using all-optical control. This switch is achieved by photochemically inducing conformational changes in the molecule. Remarkably, a Rabi splitting of 700 meV is measured at room temperature, corresponding to 32% of the molecular transition energy. A similar coupling strength is demonstrated in a plasmonic structure. Such systems present a unique combination of coupling strength and functional capacities.

U2 - 10.1103/PhysRevLett.106.196405

DO - 10.1103/PhysRevLett.106.196405

M3 - Journal article

C2 - 21668181

VL - 106

SP - 196405

JO - Physical Review - Index

JF - Physical Review - Index

SN - 0094-0003

ER -

ID: 33814946